“…19â23 Furthermore, these frameworks can be tuned by the incorporation of various heterocyclic aromatic rings, which can be coordinated to metal atoms, such as Mn. Thus, taking into account the high catalytic activities of redoxable MnO 2 nanosheets, 5 the excellent electrical conductivities of CONs, 19â23 and the synergistic hybridization effects of inorganic nanosheets on the resulting porosity, 24 the hybridization of a CON framework with ultrathin MnO 2 nanosheets would be expected to provide a powerful means to explore high-performance electrocatalyst materials via redox-induced interfacial bond formation. 6 However, at the time of this submission, we are unaware of any other work examining the redox-driven formation of strong interfacial interactions between reactive COFs and transition metal oxides as effective synthetic routes to highly efficient hybrid electrocatalysts.…”