Abstract. Using the method of offline radiative transfer modeling within the partial
radiative perturbation (PRP) approach, the effective radiative forcing
by aerosol–cloud interactions (ERFaci) in the ECHAM–HAMMOZ aerosol climate
model is decomposed into a radiative forcing by anthropogenic cloud droplet
number change and adjustments of the liquid water path and cloud fraction.
The simulated radiative forcing by anthropogenic cloud droplet
number change and liquid water path adjustment are of
approximately equal magnitude at −0.52 and
−0.53 W m−2, respectively, while the cloud-fraction adjustment is
somewhat weaker at −0.31 W m−2 (constituting 38 %, 39 %, and 23 %
of the total ERFaci, respectively); geographically, all three ERFaci components
in the simulation peak over China, the subtropical eastern ocean boundaries,
the northern Atlantic and Pacific oceans, Europe, and eastern North America (in
order of prominence). Spatial correlations indicate that the temporal-mean
liquid water path adjustment is proportional to the temporal-mean radiative
forcing, while the relationship between cloud-fraction adjustment and
radiative forcing is less direct. While the estimate of warm-cloud ERFaci is
relatively insensitive to the treatment of ice and mixed-phase cloud overlying
warm cloud, there are indications that more restrictive treatments of ice in
the column result in a low bias in the estimated magnitude of the liquid water
path adjustment and a high bias in the estimated magnitude of the droplet
number forcing. Since the present work is the first PRP decomposition of the
aerosol effective radiative forcing into radiative forcing and rapid cloud
adjustments, idealized experiments are conducted to provide evidence that the
PRP results are accurate. The experiments show that using low-frequency
(daily or monthly) time-averaged model output of the cloud property fields
underestimates the ERF, but 3-hourly mean output is sufficiently frequent.