“…The FSSH hopping probabilities are defined along each trajectory to ensure that the fraction of trajectories on each surface at any time follows the statistical populations based on wave functions. Although the FSSH results have shown good detailed balance, , the detailed internal consistency is not guaranteed due to the presence of frustrated hops and lack of decoherence. − Recently, we proposed the auxiliary branching corrected surface hopping (A-BCSH) and the auxiliary branching corrected mean field (A-BCMF) methods, which have achieved significantly better accuracy and consistency simultaneously compared to FSSH, implying a possible intrinsic connection between accuracy and detailed internal consistency in mixed quantum-classical dynamics.…”