Abstract:In strong-coupling regimes, quantum dynamical effects can alter conventional physics described by perturbation theories, but the dynamical simulations of these quantum systems using matrix product states-such as multi-level vibronic systems that are relevant to energy and electron transfer reactions-suffer from rapid entanglement growth during their real-time evolution, impeding explorations of spectra, dynamics, and kinetics. We examine the possibility of using non-unitary transformations to alter dynamical e… Show more
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.