IntroductionOur ever-increasing knowledge of light-matter interactions has enabled the development of optical components and devices for light control. These range from macroscale mirrors for the Hubble Space Telescope to nanoscale optical cavities for onchip light sources. Devices made from conventional materials, however, enable limited light manipulation. For example, the most-skilled craftsmen of conventional lenses cannot exceed the diffraction limit of light to realize subwavelength focusing.Optical metamaterials and metasurfaces of microscale or nanoscale building blocks, also known as "meta-atoms," have emerged to overcome the limits of natural materials. Due to the reduced differences in length scale between electromagnetic waves and these building blocks, metamaterials and metasurfaces enhance light-matter interactions by orders. Advancements in modeling, nanofabrication, and characterization tools [1][2][3][4][5][6][7][8] have spawned metamaterials and metasurfaces with unprecedented light-manipulation capabilities, including subwavelength focusing, negative refraction, and superabsorption. [9][10][11][12][13][14][15] Optical metamaterials and metasurfaces often rely on the strong interactions between light and meta-atoms to manipulate light-propagation properties (e.g., phase, polarization, and amplitude). With the ability of surface plasmons to concentrate light at the nanoscale, plasmonic nanostructures enhance Optical metamaterials and metasurfaces enable versatile light manipulations. Advancements in modeling, nanofabrication, and characterization tools have led to the development of metamaterials and metasurfaces for many applications: energy conversion, biomedicine, and information technology. Recently, metamaterials and metasurfaces with moiré configurations have attracted strong interest due to their highly tunable optical responses and high-throughput fabrication. Herein, state-of-the-art moiré metamaterials and metasurfaces are reviewed. The presentation covers fabrication techniques, structure-property relationships, and applications in lasing and biomedical sensing. The review concludes with challenges and opportunities for moiré metamaterials and metasurfaces. www.advopticalmat.de metasurfaces which feature microscale and nanoscale metaatoms. Next, we discuss their properties and applications. We conclude with perspectives on challenges and opportunities.