Sub-Picosecond Photodynamics of Small Neutral Copper Oxide Clusters
Chase Rotteger,
Carter Jarman,
Madison Sobol
et al.
Abstract:The ultrafast dynamics of neutral copper oxide clusters (CnOx, n < 5) are reported using femtosecond pump probe spectroscopy in the gas phase. The transient spectra recorded for each cluster demonstrates they relax on a 100s of fs timescale followed by a long-lived (>50 ps) response. Density functional theory calculations are performed to determine the lowest energy structures and spin states. Topological descripters for the excited states are calculated (time-dependent density functional theory) to rela… Show more
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