Although the modern shell-model picture of atomic nuclei is built from single-particle orbits with good total angular momentum j, leading to j-j coupling, decades ago phenomenological models suggested a simpler picture for 0p-shell nuclides can be realized via coupling of total spin S and total orbital angular momentum L. I revisit this idea with large-basis, no-core shell model (NCSM) calculations using modern ab initio two-body interactions, and dissect the resulting wavefunctions into their component L-and S-components. Remarkably, there is broad agreement with calculations using the phenomenological Cohen-Kurath forces, despite a gap of nearly fifty years and six orders of magnitude in basis dimensions. I suggest L-S decomposition may be a useful tool for analyzing ab initio wavefunctions of light nuclei, for example in the case of rotational bands.