“…In these TMDCs, the M x T S 2 (M = 3d transition metal, T = Ta, Nb) family [14] with x = 1/3 exhibit unique properties, due to the inserted ionic arranging in a stacked √ 3 × √ 3 su-perlattice, reducing the crystal symmetry. [15] For example, a chiral helical magnetic order was observed in Cr 1/3 NbS 2 , [5] a large anomalous Hall effect occurs in Co 1/3 NbS 2 . [16] In this article, on the basis of growing successfully high-quality V 1/3 TaS 2 crystals, we carried out the magnetization, longitudinal, and Hall resistivity measurements, combined with the electronic band structure calculations.…”