For each prime power q ≥ 5, we construct a rank four chiral polytope that has a group PSL(3, q) as automorphism group and Schläfli type {q − 1, 2(q−1) (3,q−1) , q − 1}. We also construct rank five polytopes for some values of q and we show that there is no chiral polytope of rank at least six having a group PSL(3, q) or PSU(3, q) as automorphism group.