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“…In the present geometry, where the localized resonances are at higher frequencies than the Rayleigh anomalies, both decreasing d and increasing a , increases their detuning and makes the interaction weaker. [ 59,60 ] This weaker interaction leads to narrower M‐SLRs, with a character that is more diffractive as opposed to the localized character due to Mie resonances. The effect of detuning is also clearly seen in the extinction maps of Figure 2, where the frequencies of the diffraction orders are tailored via the angle of incidence.…”
An enhanced emission of high quantum yield molecules coupled to dielectric metasurfaces formed by periodic arrays of polycrystalline silicon nanoparticles is demonstrated. Radiative coupling of the nanoparticles, mediated by in‐plane diffraction, leads to the formation of collective Mie scattering resonances or Mie surface lattice resonances (M‐SLRs), with remarkable narrow line widths. These narrow line widths and the intrinsic electric and magnetic dipole moments of the individual Si nanoparticles allow resolving electric and magnetic M‐SLRs. Incidence angle‐ and polarization‐dependent extinction measurements and high‐accuracy surface integral simulations show unambiguously that magnetic M‐SLRs arise from in‐ and out‐of‐plane magnetic dipoles, while electric M‐SLRs are due to in‐plane electric dipoles. Pronounced changes in the emission spectrum of the molecules are observed, with almost a 20‐fold enhancement of the emission in defined directions of molecules coupled to electric M‐SLRs, and a fivefold enhancement of the emission of molecules coupled to magnetic M‐SLRs. These measurements demonstrate the potential of dielectric metasurfaces for emission control and enhancement, and open new opportunities to induce asymmetric scattering and emission using collective electric and magnetic resonances.
“…In the present geometry, where the localized resonances are at higher frequencies than the Rayleigh anomalies, both decreasing d and increasing a , increases their detuning and makes the interaction weaker. [ 59,60 ] This weaker interaction leads to narrower M‐SLRs, with a character that is more diffractive as opposed to the localized character due to Mie resonances. The effect of detuning is also clearly seen in the extinction maps of Figure 2, where the frequencies of the diffraction orders are tailored via the angle of incidence.…”
An enhanced emission of high quantum yield molecules coupled to dielectric metasurfaces formed by periodic arrays of polycrystalline silicon nanoparticles is demonstrated. Radiative coupling of the nanoparticles, mediated by in‐plane diffraction, leads to the formation of collective Mie scattering resonances or Mie surface lattice resonances (M‐SLRs), with remarkable narrow line widths. These narrow line widths and the intrinsic electric and magnetic dipole moments of the individual Si nanoparticles allow resolving electric and magnetic M‐SLRs. Incidence angle‐ and polarization‐dependent extinction measurements and high‐accuracy surface integral simulations show unambiguously that magnetic M‐SLRs arise from in‐ and out‐of‐plane magnetic dipoles, while electric M‐SLRs are due to in‐plane electric dipoles. Pronounced changes in the emission spectrum of the molecules are observed, with almost a 20‐fold enhancement of the emission in defined directions of molecules coupled to electric M‐SLRs, and a fivefold enhancement of the emission of molecules coupled to magnetic M‐SLRs. These measurements demonstrate the potential of dielectric metasurfaces for emission control and enhancement, and open new opportunities to induce asymmetric scattering and emission using collective electric and magnetic resonances.
“…Technological flexibility in the design of plasmonic cavities allows one to engineer surface-plasmon states and their interactions with quantum emitters (QEs), e.g., fluorescent dyes or semiconductor nanostructures, leading to potentially desirable cooperative properties [1][2][3]. The strong (ultrastrong) coupling regimes, when the surface-plasmon-QE interaction strength exceeds the total cavity losses (becomes comparable to the QE energy), open new opportunities for nonequilibrium exciton-plasmon-polariton condensation, nonlinear emission, and lasing [4,5].…”
Hybrid photonic-plasmonic nanostructures allow one to engineer coupling of quantum emitters and cavity modes accounting for the direct coherent and environment-mediated dissipative pathways. Using the generalized plasmonic Dicke model, we explore the nonequilibrium phase diagram with respect to these interactions. The analysis shows that their interplay results in the extension of the superradiant and regular lasing states to the dissipative coupling regime and an emergent lasing phase without population inversion having a boundary with the superradiant and normal states. Calculated photon emission spectra are demonstrated to carry distinct signatures of these phases.
“…The strong coupling regime is attractive because in this regime the molecular energy landscape can be radically modified, the regime thus offers great opportunities to control molecular properties. [11][12][13][14] In the past, strong coupling of molecules to cavities has been explored using planar Fabry-Perot resonators, 6,15,16 single plasmonic particles, 17,18 meta-surfaces, 10,19,20 and gap plasmonic cavities, 21 among others.…”
We report strong coupling of a monolayer of J -aggregated dye molecules to the whispering gallery modes of a dielectric microsphere at room temperature. We systematically studied the evolution of strong coupling as the number of layers of dye molecules was increased, we found the Rabi splitting to rise from 56 meV for a single layer to 94 meV for four layers of dye molecules. We compare our experimental results with 2D numerical simulations and a simple coupled oscillator model, finding good agreement.We anticipate that these results will act as a stepping stone for integrating moleculecavity strong coupling in a microfluidic environment since microspheres can be easily trapped and manipulated in such an environment, and provide open access cavities.
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