2013
DOI: 10.1002/pssr.201308154
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Strain engineering of topological properties in lead‐salt semiconductors

Abstract: Rock-salt chalcogenide SnTe represents the simplest realization of a topological insulator where a crystal symmetry allows for the appearence of topologically protected metallic states with an even number of Dirac cones on high-symmetry crystal surfaces. Related rock-salt lead chalcogenides have been predicted as well to undergo a phase-transition to a topological crystalline insulating phase after band inversion induced by alloying and pressure. Here we theoretically predict that strain, as realized in thin f… Show more

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Cited by 29 publications
(27 citation statements)
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“…This causes a shift in the position of the low-energy Dirac points + and − along the mirror-symmetric line X 1 in opposite directions by an equal amount. This Dirac point shift under uniform strain, which we deduce from symmetry analysis here, has been found in recent ab initio calculations [20,21].…”
Section: B Strainsupporting
confidence: 85%
“…This causes a shift in the position of the low-energy Dirac points + and − along the mirror-symmetric line X 1 in opposite directions by an equal amount. This Dirac point shift under uniform strain, which we deduce from symmetry analysis here, has been found in recent ab initio calculations [20,21].…”
Section: B Strainsupporting
confidence: 85%
“…As mentioned by Hsieh et al 42 , with the lattice constant decreasing, PbTe can be changed from a NI to a TCI. Such topological phase transition also occurs for other lead chalcogenides under external pressure or volume compression 80,81 ; while for the volume expansion, SnS and SnSe can be transformed from an ambient pressure TCI to a topologically trivial insulator 82 .…”
Section: A Strain Effect On Bulk: Topological Phase Transitionmentioning
confidence: 82%
“…Our observations are captured by a tight binding model, and provide experimental support for the existing body of theoretical work studying the role of surface orientations in TCI materials. Finally, our demonstration of successfully growing and measuring (Pb,Sn)Se films constitutes an important step towards future studies, enabling investigations into the role of strain 25 (through lattice-mismatch from different substrates), additional surface orientations (for example the (110) facet) and atomic step density through substrate vicinality.…”
Section: Discussionmentioning
confidence: 99%