Abstract:In the orthorhombic compound holmium trifluoride, HoF,, the trivalent holmium ion has a singlet ground state, with another singlet at 5.90 cm-l. Optical spectroscopy, magnetic and thermal measurements are used to investigate the behaviour of single crystals at 4.2 K and below. The results largely confirm the crystal-field analysis of Ram and Sharma, but give a value of 6.59 cm-' for the separation of the two singlets. It is found also that the system orders antiferromagnetically at TN = 0.53 K, with the holmiu… Show more
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