2013
DOI: 10.1063/1.4807170
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Stimulated Raman scattering in the evanescent field of liquid immersed tapered nanofibers

Abstract: International audienceWe present the first experimental demonstrations of stimulated Raman scattering in a liquid probed by the evanescent field of a tapered silica nanofiber. Raman scattering by a pure liquid, ethanol, or mixture of liquids, toluene diluted in ethanol, is investigated. Given the large choice of available materials for the medium surrounding the nanofiber, these demonstrations pave the way to the exploration of a new class of experiments and devices

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Cited by 27 publications
(30 citation statements)
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“…Here we report a nanofiber (NF)-based evanescent-wave SRS spectroscopic technique for trace hydrogen detection. NFs are one of the best carriers for nonlinear light-matter interaction [14,15], and in virtue of the high light intensity in the evanescent field, the SRS efficiency of molecules around a NF could be orders of magnitude higher than in a HC-PCF. The technique has the merits of high selectivity, fast response, large dynamic range, and superior signal-to-noise ratio, enabling the best overall performance of fiber-optic hydrogen sensors to our knowledge.…”
Section: Introductionmentioning
confidence: 99%
“…Here we report a nanofiber (NF)-based evanescent-wave SRS spectroscopic technique for trace hydrogen detection. NFs are one of the best carriers for nonlinear light-matter interaction [14,15], and in virtue of the high light intensity in the evanescent field, the SRS efficiency of molecules around a NF could be orders of magnitude higher than in a HC-PCF. The technique has the merits of high selectivity, fast response, large dynamic range, and superior signal-to-noise ratio, enabling the best overall performance of fiber-optic hydrogen sensors to our knowledge.…”
Section: Introductionmentioning
confidence: 99%
“…From simulations of the Raman cascade [12] and from previous experimental studies [27] we can estimate that the temporal pulse duration at 583 nm is shorter than the pump pulse duration (i.e. 560 ps FWHM), an order of magnitude of this pulse duration at maximum pump power is expected to be around 100-200 ps FWHM by the numerical simulations.…”
Section: Resultsmentioning
confidence: 78%
“…To improve the sensitivity of these devices, the enhancement of the evanescent effect is benefit and has been usually adopted [11]. Microfibers, which possess high fraction of the evanescent wave highly sensitive to the variations of environmental parameters, are good candidates for the sensing occasions with high-sensitivity sensing with small footprint and fast response [12][13]. It is promising to integrate function materials with tapered fibers to develop fiber-based integrated photonic devices with high sensitivity.…”
Section: Introductionmentioning
confidence: 98%