The authors have investigated the use of fast neutrons-primarily the fast neutron energy spectrum-as a signature for uranium hexafluoride (UF 6 ) nuclear accountancy measurements. Detailed modeling of UF 6 storage cylinders and a proposed neutron detection system indicates that the measured neutron energy spectrum is indeed a function of uranium enrichment. Field measurements at the Department of Energy's Paducah Gaseous Diffusion Plant with a detection system similar to the modeled system provided an opportunity to collect signatures from several storage cylinders containing UF 6 with a range of enrichments. Subsequent analysis lends credibility to the modeling results, indicating that enrichment over the range measured (0.72% to 4.95% uranium-235) can be extracted from the measured neutron energy spectrum. These results were scaled to estimate the tradeoff in measurement system size and counting time to achieve a relative enrichment measurement uncertainty of 5%.
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ACKNOWLEDGMENTSThe authors would like to thank several individuals for their contributions to this project. Robert Cooper provided modeling support for the simulated emissions of 30B cylinders, and played an important role in experiments and analysis of the detector response. Laura Kogler provided important analysis support, and generated important comparisons of the Neutron Scatter Camera to other mature technologies. Isaac Shokair was very helpful in understanding implementation of the Principal Component Analysis technique. Michael Streicher provided important simulation and experimental support, which was useful in understanding the detector response to 30B emissions and the characterization of hardware in the laboratory.Jim Brennan and Dan Throckmorton provided support during the assembly of the detector system fielded at the Paducah Gaseous Diffusion Plant (PGDP). Stanley Mrowka provided software for the data acquisition system and assisted in the data collection at PGDP. Randy DeVault (DOE/Oak Ridge Field Office) and Richard Mayer (DOE/Lexington Field Office) were instrumental in identifying and facilitating the measurement opportunity at PGDP. Brent Montgomery, John Price, and Tullus Crawford of the United States Enrichment Corporation (USEC) provided support for the PGDP measurements.