State Resolved Sticking Probability in Gas-Surface Interaction

Vattuone, L.; Okada, Michio

doi:10.1007/978-3-030-46906-1_32

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2023

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“…Such theoretical work provides excellent data for comparison with surface dynamics experiments under well-controlled UHV conditions. A classical experimental approach probes the entrance channel of the reaction pathway by employing pulsed molecular beams of reactants to initiate the surface reaction ( Barker and Auerbach, 1984 ; Kleyn et al, 1996 ; Sitz, 2002 ; Kleyn, 2003 ; Golibrzuch et al, 2015 ; Chadwick and Beck, 2016 ; Vattuone and Okada, 2020 ; Shen et al, 2022 ). Seeding reactants in different carrier gases allows for modification of the incident translational energy.…”

Section: Introductionmentioning

confidence: 99%

Hyperthermal velocity distributions of recombinatively-desorbing oxygen from Ag(111)

Dorst,

Dissanayake,

Schauermann

et al. 2023

Front. Chem.

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This study presents velocity-resolved desorption experiments of recombinatively-desorbing oxygen from Ag (111). We combine molecular beam techniques, ion imaging, and temperature-programmed desorption to obtain translational energy distributions of desorbing O2. Molecular beams of NO2 are used to prepare a p (4 × 4)-O adlayer on the silver crystal. The translational energy distributions of O2 are shifted towards hyperthermal energies indicating desorption from an intermediate activated molecular chemisorption state.

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