We propose a protocol to create maximally entangled pairs, triplets, quartiles, and other clusters of Bose condensed atoms starting from a condensate in the Mott insulator state. The essential element is to drive single atom Raman transitions using laser pulses. Our scheme is simple, efficient, and can be readily applied to the recent experimental system as reported by Greiner et al. [ Nature 413, 44 (2002)].03.65. Ud, 03.75.Fi The physics of quantum degenerate atomic gases continues in its rapid pace of development, and remains one of the most active research areas in recent years [1]. Increasingly, theoretical and experimental attentions are directed towards the underlying quantum correlation properties of the condensed atoms. It seems likely that such quantum states of matter might prove to be a fertile ground for exploring quantum information science applications.Recently, a quantum phase transition was observed in a system of Bose condensed atoms immersed in a periodic array of optical potentials [2]. As expected, when expressed in the simple Bose-Hubbard form [3], the ground state of such a system is controlled by essentially two parameters: 1) the on-site atom-atom interaction u for atoms in the same spatial mode of each individual optical well; and 2) the nearest neighboring well (single) atom tunnelling rate J (taken as positive). When J ≫ |u|, the condensate ground state is in the usual superfluid (delocalized single atom) state. On the other hand, a Mott insulator state arrives in the opposite limit |u| ≫ J. In a Mott state, atoms are localized inside individual wells. The condensate ground state takes the form of a product of Fock states with an integer number of atoms on each site. The transition from superfluid to Mott insulator is predicted to occur at |u|/J ≥ z × 2.6 with z the number of nearest neighbors in the periodic well lattice [3,4].The experimental system that yielded the first clear demonstration of the superfluid/Mott-insulator transition enables individual tuning of the values for both J and u [2]. In the experiment, the average occupations per well was around 1-3 atoms, which could potentially form elementary building blocks for atomic qubit based quantum computing designs [3].In this paper, we propose to create massive maximum entangled pairs, triplets, quartiles, and other clusters of Bose condensed atoms in a Mott insulator state. The resulting entanglement, with respect to electronic internal states, is stable and long lived. In the experiment [2] 87 Rb atoms in the magnetic trapping state |a = |F = 2, M F = −2 were used. Other internal states can be trapped in the same experimental setup. In the simple model to be presented below, a second internal state |b that can be coupled to |a through atomic Raman transitions is assumed [2] (as see earlier JILA experiments with 87 Rb states |F = 2, M F = −1 andIn a Mott state, the system dynamics is rather simple as there exists a fixed (small) number of atoms within each well. If we use the second quantized operators a(a † ) and b(b † )...