2014
DOI: 10.1021/jp5059947
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Spin-Polarized Negative Differential Resistance in a Self-Assembled Molecular Chain

Abstract: By using first-principles calculations, we investigate the electronic structures and transport properties of a self-assembled Fe 2 −PTCDA chain. This experimentally observed chain can grow as long as a few tens of nanometers and our calculations suggest that it conducts as a half-metal. Spin-polarized transport properties are attributed to conducting bands of the minority spin near the Fermi energy, raised by the hybridization between orbitals of the molecule and the iron atoms, while a band gap of the majorit… Show more

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Cited by 10 publications
(4 citation statements)
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“…In this work, we reported the spin-dependent negative differential resistance (SPNDR) in DNA by studying the I – V characteristic for spin current (Figure ). This effect is experimentally reported in a self-assembled molecular chain and graphene nanoribbons previously. An SPNDR device will enrich spintronics as well.…”
Section: Resultssupporting
confidence: 78%
“…In this work, we reported the spin-dependent negative differential resistance (SPNDR) in DNA by studying the I – V characteristic for spin current (Figure ). This effect is experimentally reported in a self-assembled molecular chain and graphene nanoribbons previously. An SPNDR device will enrich spintronics as well.…”
Section: Resultssupporting
confidence: 78%
“…It shows that only the spin-up channel can produce the current, whereas the current of the spin-down channel is equal to zero, implying that the current in the 1D CrN is 100% spin-polarized. More interestingly, the characteristic of negative differential resistance (NDR) [42][43][44] can be observed when the voltage is larger than 1.0 V. By analyzing the transmission spectra in Figs. 4(b) and 4(c), we find that with the increase of bias voltage, although the bias energy window becomes wider, the transmission inside the window is suppressed, which di-rectly results in the occurrence of NDR phenomenon.…”
Section: Resultsmentioning
confidence: 99%
“…Such regions are known as spin-dependent negative differential resistance (SPNDR) areas. SPNDR is experimen- tally demonstrated in a self-assembled molecular chain 40 and theoretically in DNA-based materials. 18 An SPNDR device enhances spintronic devices.…”
Section: ■ Methodsmentioning
confidence: 99%