For advanced quantum information technology, sources of photon pairs in quantum mechanically factorable states are of great importance for realizing high-fidelity photon-photon quantum gate operations. Here we experimentally demonstrate a technique to produce spectrally factorable photon pairs utilizing multi-order quasi-phase-matching (QPM) conditions in spontaneous parametric downconversion (SPDC). In our scheme, a spatial nonlinearity profile of a nonlinear optical crystal is shaped with current standard poling techniques, and the associated phase-matching function can be approximated to a Gaussian form. By the measurement of a phase-matching function and the second-order autocorrelation function, we demonstrate that telecom-band photon pairs produced by our custom-poled crystal are highly factorable with > 95% single-photon purity.
I. INTRODUCTIONQuantum photonics technology plays an important role in various quantum applications such as quantum computing [1, 2], quantum communication [3,4], quantum metrology [5], and bridging solid and atomic quantum systems at a distance [6]. One of the central requirements in the quantum photonics technology is to produce pure single photons. Most multi-photon applications rely on interference of independent single photons [7], and only pure and indistinguishable photons can exhibit perfect interference. Photon-pair generation via spontaneous parametric downconversion (SPDC) has been widely accepted in quantum optics and photonic quantum information experi-