Efficient detection of ionizing radiation plays a central role in several scientific and technological fields such as high energy and particle physics, astronomy, geology, medical diagnostics, nuclear monitoring, oil extraction, and space exploration. [1] In all such areas the most widely used detectors are scintillating materials that convert the energy deposited by incoming ionizing radiation into visible photons, which are then turned into electrical signals by coupled photodetectors (e.g. photomultiplier tubes or silicon photomultipliers). [2] The relatively simple device architecture and the availability of high atomic number (Z) materials efficiently interacting with ionizing radiation of various energies (the interaction probability scales with Z n with n = 1-5 depending on the interaction mechanism [1f,3] ) is enabling rapid progress in the design of scintillators optimized for specific application requirements. [4] A valuable class of radiation detectors is represented by plastic scintillators that can be produced in large sizes not achievable with inorganic single crystals, low weight, and affordable costs that make them particularly suitable for radiation monitoring in border and industrial control. [2b,5] However, being constituted of light organic materials, plastic scintillators typically suffer from relatively low density that limits their interaction with ionizing radiation and therefore require doping with high-Z components, such as organometallic complexes or nanoparticles containing heavy elements. [2b,6] Amongst the various systems proposed to date, direct bandgap colloidal semiconductor nanocrystals (NCs) featuring efficient excitonic photophysics, such as cadmium or zinc chalcogenides or lead halide perovskites, are gaining particular interest as nanoscintillators, as they both enhance the interaction probability with ionizing radiation and effectively convert the deposited energy into visible light whose wavelength can be finely tuned by size and composition control. [2b,7] Furthermore, NCs also feature a rich surface chemistry [8] that enables their post-synthesis functionalization with molecular ligands that prompt their compatibility with plastic matrices, thus enabling the realization of Plastic scintillators are gaining attention as alternatives to inorganic scintillator crystals owing to their low fabrication cost, customable shape/size, and substantially lighter weight that make them suitable for various radiation detection technologies. These include scintillation panels for national security and industrial monitoring, radiation screens for medical diagnostics, and calorimeters for high energy physics. Because of their low density, plastic scintillators are typically doped with high atomic number (Z) sensitizers that enhance the interaction probability with ionizing radiation and excite molecular emitters. Although effective, such a two-component design suffers from incomplete sensitization, intrinsically limited efficiency due to multiple radiative steps with non-unity quan...