2021
DOI: 10.1039/d1ee02018h
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Solution-processed perovskite thin-films: the journey from lab- to large-scale solar cells

Abstract: This review explores perovskite crystallization in scalable deposition techniques, including blade, slot-die, spray coating, and inkjet printing.

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Cited by 127 publications
(113 citation statements)
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“…Perovskite solar cells (PSCs) have attracted enormous interest due to their rapid progress in power conversion efficiencies (PCEs) from 3.8% 1 to 25.5%. 2 To date, most PSCs with the highest PCEs are fabricated in the n-i-p structure, using a mesoporous TiO 2 layer as the electron transporting layer (ETL), [3][4][5][6] which, however, requires a high-temperature sintering process. In addition, PSCs employing TiO 2 ETLs are potentially unstable under ultraviolet (UV) illumination 7,8 and prolonged forward bias.…”
Section: Introductionmentioning
confidence: 99%
“…Perovskite solar cells (PSCs) have attracted enormous interest due to their rapid progress in power conversion efficiencies (PCEs) from 3.8% 1 to 25.5%. 2 To date, most PSCs with the highest PCEs are fabricated in the n-i-p structure, using a mesoporous TiO 2 layer as the electron transporting layer (ETL), [3][4][5][6] which, however, requires a high-temperature sintering process. In addition, PSCs employing TiO 2 ETLs are potentially unstable under ultraviolet (UV) illumination 7,8 and prolonged forward bias.…”
Section: Introductionmentioning
confidence: 99%
“…ions,p olymers,a nd solvent molecules,t oa chieve the lowtemperature crystallization of black phase inorganic perovskites,e specially with the composition CsPbI 3 .I ng eneral, low-temperature crystallization is critical for the fabrication of next-generation perovskite optoelectronics.T his includes applications of large-scale modules, [7,120,121] flexible devices, [122,123] and multijunction tandem photovoltaics. [74,124,125] Fort he fabrication of large-area solar cell modules,alow crystallization temperature of the perovskite layer can ease the manufacturing process and reduce the cost for industrialization.…”
Section: Methodsmentioning
confidence: 99%
“…Lead halide perovskites have excellent optoelectronic properties, such as a high absorption coefficient, high carrier mobility, and long carrier recombination life. Due to these excellent properties, the PCE of perovskite solar cells (PSCs) achieved an explosive development from 3.8% to 25.7% in a few years [1][2][3][4][5][6]. Despite the advance in the PCE of PSCs, the moisture instability of the perovskite layer, under ambient conditions, is one of the most urgent problems to be resolved.…”
Section: Introductionmentioning
confidence: 99%