2021
DOI: 10.1002/ange.202111285
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Solid‐State Red Laser with a Single Longitudinal Mode from Carbon Dots

Abstract: Miniaturized solid‐state lasers with a single longitudinal mode are vital for various photonic applications. Here we prepare red‐emissive carbon dots (CDs) with a photoluminescence quantum yield (PLQY) of 65.5 % by combining graphitic nitrogen doping and surface modification. High‐concentration doping alters the CDs’ emission from blue to red, while the electron‐donating groups and polymer coating on their surfaces improve the PLQY and photostability. The CDs exhibit excellent stimulated emission characteristi… Show more

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Cited by 9 publications
(3 citation statements)
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“…The absorption peak at 1610–1635 cm –1 is due to the stretching vibration of OC–N and OC–O. The characteristic absorption peaks located at 1574, 1400, and 1055 cm –1 originate from the characteristic vibration peak of the benzene ring, deformed vibration of C–N, and stretching vibration of C–O. FT-IR results were confirmed by the XPS deconvolution spectra. As Figure B–D shows, the C 1s image proves the existence of CC/C–C (284.6 eV), C–N/C–O (285.9 eV), and OC–N/OC–O (289.9 eV).…”
Section: Resultsmentioning
confidence: 57%
“…The absorption peak at 1610–1635 cm –1 is due to the stretching vibration of OC–N and OC–O. The characteristic absorption peaks located at 1574, 1400, and 1055 cm –1 originate from the characteristic vibration peak of the benzene ring, deformed vibration of C–N, and stretching vibration of C–O. FT-IR results were confirmed by the XPS deconvolution spectra. As Figure B–D shows, the C 1s image proves the existence of CC/C–C (284.6 eV), C–N/C–O (285.9 eV), and OC–N/OC–O (289.9 eV).…”
Section: Resultsmentioning
confidence: 57%
“…As a new type of carbon-based fluorescent nanomaterial, CDs have recently received extensive research attention for their diverse physicochemical properties, abundant surface groups (such as amino, carboxyl, and hydroxyl groups, etc. ), environmental friendliness, and low cost. Among them, simple preparation methods, high PLQY, low toxicity, and tunable emission spectra are considered by researchers as the ideal luminophores in LSCs. , …”
Section: Single-layer Lscsmentioning
confidence: 99%
“…13 A SiO 2 -CDots thin film (emitting at 588 nm) and SiO 2 -CDots powder (emitting at 597 nm) were obtained by physically embedding CDots into a silicon dioxide matrix. 7 Furthermore, dual-wavelength emitting solid-state CDots have been developed owing to their great potential applications in storage 17,18 and solid-state lasing, 19 and photonic and lightconverting devices, which require broad emission covering the whole visible region. 20 For instance, the dual-emission solidstate CDots with the wavelengths of 410 nm and 500 nm by the matrices of Na ions.…”
Section: Introductionmentioning
confidence: 99%