1969
DOI: 10.1016/0022-3115(69)90124-x
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Solid fission product behavior in uranium-plutonium oxide fuel irradiated in a fast neutron flux

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Cited by 82 publications
(18 citation statements)
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“…The maximum solubility of SrO in UO 2 was experimentally 95 found to be much higher in UO 2 than in UO 2-x , which mirrors our calculated trend. This can be explained on the fact that the solution of strontium becomes increasingly favorable as one approaches hyperstoichiometric conditions owing to the strong Coulombic interactions.…”
Section: +supporting
confidence: 90%
See 1 more Smart Citation
“…The maximum solubility of SrO in UO 2 was experimentally 95 found to be much higher in UO 2 than in UO 2-x , which mirrors our calculated trend. This can be explained on the fact that the solution of strontium becomes increasingly favorable as one approaches hyperstoichiometric conditions owing to the strong Coulombic interactions.…”
Section: +supporting
confidence: 90%
“…Considering individual oxides, Cs 2 O is predicted to be stable at all stoichiometries, though in UO 2+x , it is on the borderline of stability. With regard to UO 2+x , it is also observed experimentally 95 that the solubility of Cs increases as we go from hypostoichiometric to hyperstoichiometric fuels. Our calculations support this argument.…”
Section: +mentioning
confidence: 76%
“…No melting [6] center of the pellet leaves a more fully dense fuel material behind and this can result in a large hole in the center of the pellet. Most of this restructuring occurs in a matter of hours at full power.…”
Section: Fig 85mentioning
confidence: 98%
“…It has smaller diameter pins (5.8 mm) than a typical power SFR. 6 Pores are tiny void spaces purposely fabricated into the fuel to allow space for fuel swelling and expansion during steady-state and thermal upset conditions. Porosity is the fraction of the fuel volume that is void.…”
Section: Fuel Restructuringmentioning
confidence: 99%
“…Cesium and molybdenum can be soluble or insoluble depending on conditions, most notably the oxygen activity. [1][2][3] Consequently, voids, gas bubbles, second phases, and new compounds are formed continuously during the service life of the pellet, and during post-service storage. To add further complexity, pellet-clad interactions can lead to additional chemical changes in the fuel.…”
Section: Introductionmentioning
confidence: 99%