2Due to the intrinsic isotropic magnetic properties, soft magnetic composite (SMC) materials are applied in electrical machines in which the magnetic energy can be transported in three dimensional (3-D). However, in real application, complicated magnetic properties, such as anisotropy and nonlinearity, are found, in particular, at the high frequency range. This paper studies the 3-D magnetic properties of SMC materials under complicated magnetization, such as circular, elliptical, and spherical excitations. The magnetic flux density vector B loci and magnetic field strength vector H loci and core losses at magnetization frequencies ranged from 50 Hz to 1000 Hz were measured and discussed using an improved 3-D testing system. Experimental results show that rotational core losses are greater than alternating losses at the same magnitude of flux density. In addition, rotational loss increases sharply after saturation point, but it is not observed in alternating loss.3