Abstract:Optical gas detection in microsystems is limited by the short micron scale optical path length available. Recently, the concept of slow-light enhanced absorption has been proposed as a route to compensate for the short path length in miniaturized absorption cells. We extend the previous perturbation theory to the case of a Bragg stack infiltrated by a spectrally strongly dispersive gas with a narrow and distinct absorption peak. We show that considerable signal enhancement is possible. As an example, we consid… Show more
“…Recent works [7,8] have theoretically demonstrated that Beer-Lambert-Bouguer (BLB) absorption can be increased while light transmits through a special kind of microstructured photonic crystal (PC) cuvette. This absorption enhancement was attributed in [7,8] to the slow group velocity in the cuvette. A simpler interpretation of these results would be that the PC structure acts as a quasi-cavity.…”
We experimentally demonstrate that material slow light does not enhance Beer-Lambert absorption. A 26% group velocity reduction induced by stimulated Brillouin scattering in a gasfilled microstructured fiber caused no observable change in the measured absorption.
“…Recent works [7,8] have theoretically demonstrated that Beer-Lambert-Bouguer (BLB) absorption can be increased while light transmits through a special kind of microstructured photonic crystal (PC) cuvette. This absorption enhancement was attributed in [7,8] to the slow group velocity in the cuvette. A simpler interpretation of these results would be that the PC structure acts as a quasi-cavity.…”
We experimentally demonstrate that material slow light does not enhance Beer-Lambert absorption. A 26% group velocity reduction induced by stimulated Brillouin scattering in a gasfilled microstructured fiber caused no observable change in the measured absorption.
“…Since the dependence of the optical absorption of molecules on the group velocity is radically different depending on the slowlight generation mechanism, this clarifies that the group velocity is not the appropriate universal quantity scaling lightmatter interactions. In a periodic, lossless media such as ring resonators the velocity of energy propagation is identical to the group velocity of a quasi-monochromatic wave [14][15][16][17][18] [8,9]. Reducing the electromagnetic energy velocity through structural slow light effectively increases the electromagnetic energy density and yields the observed enhancement of light-matter interactions.…”
Section: Discussionmentioning
confidence: 99%
“…The role of slow light in gyroscopes has also been theoretically investigated 5 and the possibility to use fiber Bragg gratings to realize ultrasensitive strain sensors has been experimentally proved 6 . Recent works 7,8 have theoretically demonstrated that BeerLambert-Bouguer (BLB) absorption can be increased while light transmits through a special kind of microstructured photonic crystal (PC) cuvette. This absorption enhancement was attributed in these works 7,8 to the slow group velocity in the cuvette.…”
Section: Introductionmentioning
confidence: 99%
“…Recent works 7,8 have theoretically demonstrated that BeerLambert-Bouguer (BLB) absorption can be increased while light transmits through a special kind of microstructured photonic crystal (PC) cuvette. This absorption enhancement was attributed in these works 7,8 to the slow group velocity in the cuvette. A simpler interpretation of these results would be that the PC structure acts as a quasi-cavity.…”
A couple of experiments are here presented to clarify the impact of slow light on light-matter interaction. The experiments are designed, so that the process generating slow light and the probed light-matter interaction only present a marginal cross-effect. The impact of slow light on simple molecular absorption could be separately evaluated under either material or structural slow light propagation in the same medium and led to an entirely different response.
“…A one-dimensional Bragg stack [8] is one example of a structure that can enhance the net absorption experienced by a beam traversing the structure. In this case, the picture of a beam propagation path that is effectively prolonged by multiple back-and-forth scattering in the propagation direction offers a simple physical interpretation.…”
Light traversing a hollow-core photonic band-gap fiber may experience multiple reflections and thereby a slow-down and enhanced optical path length. This offers a technologically interesting way of increasing the optical absorption of an otherwise weakly absorbing material which can infiltrate the fibre. However, in contrast to structures with a refractive index that varies along the propagation direction, like Bragg stacks, the translationally invariant structures studied here feature an intrinsic trade-off between light slow-down and filling fraction that limits the net absorption enhancement. We quantify the degree of absorption enhancement that can be achieved and its dependence on key material parameters. By treating the absorption and index on equal footing, we demonstrate the existence of an absorption-induced saturation of the group index that itself limits the maximum absorption enhancement that can be achieved.
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