Nowadays, wearable electronic devices are developing
rapidly with
the internet of things and human–computer interactions. However,
there are problems such as low power, short power supply time, and
difficulty in charging, leading to a limited range of practical applications.
In this paper, a composite hydrogel composed of polyacrylamide, hydroxypropyl
methylcellulose, and MXene (Ti3C2T
x
) nanosheets was developed, which formed a stable
double-chain structure by hydrogen bonding. The configuration endows
the hydrogel with excellent properties, such as high strength, strong
stretchability, excellent electrical conductivity, and high strain
sensitivity. Based on these characteristics, a flexible multifunctional
triboelectric nanogenerator (PHM–TENG) was prepared using the
hydrogel as a functional electrode. The nanogenerator can collect
biomechanical energy and convert it to 183 V with a maximum power
density of 78.3 mW/m2. It is worth noting that PHM–TENG
can be applied as a green power source for driving miniature electronics.
Also, it can be used as an auto-powered strain sensor that distinguishes
letters, enabling monitoring under small strain conditions. This work
is anticipated to provide an avenue for the development of new intelligent
systems for handwriting recognition.