2020
DOI: 10.26434/chemrxiv.12416042.v2
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Simultaneous Suppression of pi- and sigma- Transmission in pi-Conjugated Molecules

Abstract: <div><div><div><p>Molecular dielectric materials require ostensibly conflicting requirements of high polarizability and low conductivity. As previous efforts towards molecular insulators focused on saturated molecules, it remains an open question whether pi- and sigma-transport can be simultaneously suppressed in conjugated systems. Here, we demonstrate that there are conjugated molecules where the sigma-transmission is suppressed by destructive sigma-interference, while the pi-transmis… Show more

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