“…Relative to light intensity measurements, optical measurements that include polarization analysis have a higher dimensionality of information, and high-dimensional polarization data convey rich optical properties of particles including composition, refractive index, particle size distribution, and morphology characteristics, which allow for more accurate aerosol classification and enhance the ability to identify mixed aerosols 12,13 . This paper takes five types of natural samples, including motor vehicle exhaust, blind coal, coal, biomass combustion and dust, which are common pollutants in urban development, as an example, and focuses on the application of distribution spectra and central spectra of multidimensional polarization metrics in the classification and resolution of mixed aerosols.…”