Simultaneous Physical Cross-Linking and Mechanical Strengthening of Elastomers by Enantiomeric Interactions through Reactive Processing
Yihang Chen,
Xiayan Ling,
Jiali Wu
et al.
Abstract:Exploiting robust elastomers without sacrificing thermoplasticity has been extremely desired for decades, yet it is challenging. Noncovalent interactions are a versatile platform for the development of networks with reversible cross-linking joints. Herein, an alternative strategy is proposed to straightforwardly construct a mechanical strengthening elastomer with a dynamic cross-linking network via multiple H-bonding between enantiomeric polymer pairs. First, poly-L-lactic acid (PLLA)/poly-D-lactic acid (PDLA)… Show more
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