Simplifying tailored generation of complex structured femtosecond pulses with easily fabricated phase plates

Abstract

This article presents a novel approach to targeted 4f pulse shaping using phase plates fabricated by single-point diamond turning (SPDT) machining. The manufacturing of the phase plates using SPDT is versatile, cost-effective, fast, robust, and applicable across a wide range of optical materials, spanning from visible to far-infrared spectra (e.g., PMMA, ZnSe). Manufactured profiles can be used for phase manipulation and pulse structuring, analogously to programable spatial light modulators (SLM). We demonstrate that the pulse waveforms can be reproduced with high fidelity by simple simulations based on calculating optical path differences induced by the phase plate for each wavelength and taking into account the finite focal spot. The simulated and reconstructed frequency-resolved optical gating spectrograms featured G errors between 1–2% and intensity errors between 0.02–0.06. Even for complex structured pulses with the rms value of the time-bandwidth product reaching 12, our method maintains high precision, in some cases even reaching lower G error compared to simpler waveforms. Finally, we also show that the phase plate can be used to attain a set of uncorrelated pulse waveforms by moving the plate relatively to the dispersed laser spectrum. Overall, this approach bypasses common limitations associated with pulse shaping using SLMs, such as pixelation, pixel cross-talk, and spectral or laser fluences constraints.