Atmospheric flows exhibit self-similar fractal space-time fluctuations on all space-time scales in association with inverse power law distribution for power spectra of meteorological parameters such as wind, temperature, etc., and thus implies long-range correlations, identified as self-organized criticality generic to dynamical systems in nature. A general systems theory based on classical statistical physical concepts developed by the author visualizes the fractal fluctuations to result from the coexistence of eddy fluctuations in an eddy continuum, the larger scale eddies being the integrated mean of enclosed smaller scale eddies. The model satisfies the maximum entropy principle and predicts that the probability distributions of component eddy amplitudes and the corresponding variances (power spectra) are quantified by the same universal inverse power law distribution which is a function of the golden mean. Atmospheric particulates are held in suspension by the vertical velocity distribution (spectrum). The atmospheric particulate size spectrum is derived in terms of the model predicted universal inverse power law characterizing atmospheric eddy spectrum. Model predicted spectrum is in agreement with the following four experimentally determined data sets: (i) CIRPAS mission TARFOX_WALLOPS_SMPS aerosol size distributions (ii) CIRPAS mission ARM-IOP (Ponca City, OK) aerosol size distributions (iii) SAFARI 2000 CV-580 (CARG Aerosol and Cloud Data) cloud drop size distributions and (iv) TWP-ICE (Darwin, Australia) rain drop size distributions.Key words: universal spectrum for atmospheric suspended particulates, fractal fluctuations in atmospheric flows, chaos and nonlinear dynamics, TARFOX and ARM-IOP aerosol size spectra, SAFARI 2000 cloud drop size spectra, TWP-ICE (Darwin, Australia) rain drop size spectra.
Atmospheric suspended particulates: current state of knowledge 2.1 Aerosol size distributionAs aerosol size is one of the most important parameters in describing aerosol properties and their interaction with the atmosphere, its determination and use is of fundamental importance. Aerosol size covers several decades in diameter and hence a variety of instruments are required for its determination. This necessitates several definitions of the diameter, the most common being the geometric diameter d. The size fraction with d > 1-2 μm is usually referred to as the coarse mode, and the fraction d < 1-2 μm is the fine mode. The latter mode can be further divided into the accumulation d ~ 0.1-1 μm, Aitken d ~ 0.01-0.1 um, and nucleation d < 0.01μm modes. Due to the d 3 dependence of aerosol volume (and mass), the coarse mode is typified by a maximum volume concentration and, similarly, the accumulation