2014
DOI: 10.1021/am5054338
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Self-Powered Ultrafast Broadband Photodetector Based on p–n Heterojunctions of CuO/Si Nanowire Array

Abstract: A new self-powered broadband photodetector was fabricated by coating an n-silicon nanowire (n-Si NW) array with a layer of p-cupric oxide (CuO) nanoflakes through a new simple solution synthesis method. The p-n heterojunction shows excellent rectification characteristics in the dark and distinctive photovoltaic behavior under broadband light illumination. The photoresponse of the detector at zero bias voltage shows that this self-powered photodetector is highly sensitive to visible and near-infrared light illu… Show more

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Cited by 253 publications
(120 citation statements)
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“…This observation is consistent with the fact that the charge carrier photogeneration efficiency is proportional to the absorbed photon flux. The nonlinear relationship for the variation of photocurrent against irradiance intensity can be fitted by the power law Iph=APθwhere A is a constant for a certain wavelength, and the exponent (0.5 < θ < 1) determines the response of the photocurrent to light intensity. By fitting the curves in Figure d–f with this equation, the values of θ are calculated to be 0.94, 0.95, and 0.85 at wavelengths of 620, 450, and 350 nm, respectively.…”
Section: Resultsmentioning
confidence: 99%
“…This observation is consistent with the fact that the charge carrier photogeneration efficiency is proportional to the absorbed photon flux. The nonlinear relationship for the variation of photocurrent against irradiance intensity can be fitted by the power law Iph=APθwhere A is a constant for a certain wavelength, and the exponent (0.5 < θ < 1) determines the response of the photocurrent to light intensity. By fitting the curves in Figure d–f with this equation, the values of θ are calculated to be 0.94, 0.95, and 0.85 at wavelengths of 620, 450, and 350 nm, respectively.…”
Section: Resultsmentioning
confidence: 99%
“…These four parameters can be expressed using the following equations 40, 41 : where I P is the generated photocurrent in the device, A is the area of ZnS nanotubes and P is the power of the incident illumination, , η is is the effective photocarrier generation efficiency (which is assumed to be 0.7 in our work, when taking the scattering, reflection, and incomplete absorption into consideration), h is Planck’s constant, υ is the frequency of the incident light, e is the elementary charge. At self-powered mode with the bias of 0 V, the calculated values in air of R λ  = 2.56 A/W, G  = 13.6, D*  = 1.67 × 10 10  cm Hz 1/2 W −1 and S  = 19172, respectively (Fig.…”
Section: Resultsmentioning
confidence: 99%
“…When a photodetector works in a zero external bias mode, we call it as self-driven photodetector in this paper. [11,12] Among various types of photodetectors, photodiode-based self-driven photodetectors have the special advantage of high detectivity for weak signals based on the low dark current as no external bias voltage is needed for the self-driven operation condition.…”
Section: Introductionmentioning
confidence: 99%