Selective electrosynthesis of platform chemicals from the electrocatalytic reforming of biomass-derived hexanediol

Liao, Yihuan; Huang, Shih-Ching; Lin, Chung‐Yen

doi:10.1039/d3fd00073g

Faraday Discuss.

2023

DOI: 10.1039/d3fd00073g

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Selective electrosynthesis of platform chemicals from the electrocatalytic reforming of biomass-derived hexanediol

Yihuan Liao

Shih-Ching Huang

Chung‐Yen Lin

Abstract: 6-hydroxyhexanoic acid and adipic acid are platform chemicals and are widely used as building blocks for the synthesis of important polymers. Nevertheless, the industrial syntheses of these two chemicals are...

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Cited by 3 publications

References 26 publications

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Aqueous Electrocatalytic Reduction as a Low‐Carbon and Green Route for Chemical Synthesis and Environmental Remediation

Sari,

Lin

2024

ChemElectroChem

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The green electricity‐driven electrocatalytic reduction of organic compounds in aqueous solution has merged as a sustainable and green platform for organic electrosynthesis, upcycling of chemical waste, and environmental remediation. Compared with the thermocatalytic hydrogenation process, the electrocatalytic reduction of organic compounds uses water as a proton source, which enables its operation at ambient conditions with simplified reaction schemes and significantly reduces operation cost and energy consumption. Most studies have demonstrated the development of electrocatalysts to boost the current efficiency, conversion, and product selectivity of the electrocatalytic reduction processes. Still, little attention has been paid to the mechanism (e. g., electron/proton transfer route) and related energetics behind the electrocatalytic reduction process. This Concept overviews the recent development of the electrocatalytic reduction systems for environmental remediation, pollutant upcycling, and valorization of biomass‐derived chemicals. This Concept highlights the underlying mechanisms and aims to provide instructive guidance on designing efficient and selective electrocatalytic systems.

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Aqueous Electrocatalytic Reduction as a Low‐Carbon and Green Route for Chemical Synthesis and Environmental Remediation

Sari,

Lin

2024

ChemElectroChem

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Electroactive heterojunctions of iron-based compounds in oxygen evolution reaction—Insight into synergy and mechanism

Dymerska,

Wenelska,

Zinnatullin

et al. 2024

Electrochimica Acta

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Efficient and selective electrosynthesis of 4-aminophenol at circumneutral pH from the electrocatalytic reduction of nitrophenol over the nickel-iron phosphide modified electrode

Ong,

Huang,

Lin

et al. 2023

Materials Today Sustainability

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Selective electrosynthesis of platform chemicals from the electrocatalytic reforming of biomass-derived hexanediol

Abstract: 6-hydroxyhexanoic acid and adipic acid are platform chemicals and are widely used as building blocks for the synthesis of important polymers. Nevertheless, the industrial syntheses of these two chemicals are...

Cited by 3 publications

References 26 publications

Aqueous Electrocatalytic Reduction as a Low‐Carbon and Green Route for Chemical Synthesis and Environmental Remediation

Aqueous Electrocatalytic Reduction as a Low‐Carbon and Green Route for Chemical Synthesis and Environmental Remediation

Electroactive heterojunctions of iron-based compounds in oxygen evolution reaction—Insight into synergy and mechanism

Efficient and selective electrosynthesis of 4-aminophenol at circumneutral pH from the electrocatalytic reduction of nitrophenol over the nickel-iron phosphide modified electrode

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