“…• destructive radiochemical analysis of fuel samples for direct measurement of a subset of nuclide compositions [3], • nondestructive measurements, such as gamma spectrometry or neutron counting, to measure a subset of nuclide compositions or infer fuel properties [4], and • fuel burnup simulations performed using assembly design and reactor operating information acquired from the operator [5], or a combination of the above techniques. Destructive radiochemical assay (DA) analysis of the spent fuel (usually on the scale of a fuel pellet) represents a high-accuracy method for spent fuel characterization, in which the fuel contents are measured directly, independent of any operator information.…”