2021
DOI: 10.1021/acsphotonics.1c00609
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Scalable Nanoimprint Lithography Process for Manufacturing Visible Metasurfaces Composed of High Aspect Ratio TiO2 Meta-Atoms

Abstract: We report a one-step additive manufacturing process to fabricate metalenses for visible wavelengths. Nanostructures with aspect ratios larger than eight and critical dimensions smaller than 60 nm were produced using nanoimprint lithography and a titanium dioxide nanocrystal-based imprint material, resulting in inorganic structures exhibiting a refractive index of n = 1.9. As a demonstration, we fabricate metalenses with numerical apertures (NAs) of 0.2 and focusing efficiencies over 50%. Manufacturability was … Show more

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Cited by 77 publications
(67 citation statements)
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“…Hence, the lower resolution is acceptable. Mass production of metalenses has been demonstrated by stepper/scanner lithography 53,131,[204][205][206][207][208] and nanoimprint lithography (NIL) 62,[209][210][211] technologies (Table 2), which are the most promising candidates to move metalenses from lab to fab in the future. For example, 1-cmdiameter all-glass metalenses operating at visible wavelength are manufactured using 248-nm deep-ultraviolet (DUV) projection stepper lithography 204 .…”
Section: Scaling Up and Manufacturingmentioning
confidence: 99%
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“…Hence, the lower resolution is acceptable. Mass production of metalenses has been demonstrated by stepper/scanner lithography 53,131,[204][205][206][207][208] and nanoimprint lithography (NIL) 62,[209][210][211] technologies (Table 2), which are the most promising candidates to move metalenses from lab to fab in the future. For example, 1-cmdiameter all-glass metalenses operating at visible wavelength are manufactured using 248-nm deep-ultraviolet (DUV) projection stepper lithography 204 .…”
Section: Scaling Up and Manufacturingmentioning
confidence: 99%
“…For example, thermal NIL 212 , which is widely used, requires high pressure and temperature that easily cause damage to the template and adhesive layer. UV-NIL [209][210][211] is performed at low pressures and room temperature, minimizing magnification and distortion errors. Nevertheless, the difficultly discharged bubbles in the UV curable resist cause defects in the meta-atoms.…”
Section: Scaling Up and Manufacturingmentioning
confidence: 99%
“…This will expand the handled substrate size from a chip scale to a wafer scale for further work. [ 44 ]…”
Section: Discussionmentioning
confidence: 99%
“…[ 44 ] It is partially due to the difficulty in fabricating low loss materials and demonstrating ground‐breaking applications such as “perfect lens”, and, meanwhile, “metalens” consisting of millions of meta‐atoms with nanoimprint lithography process has been successfully demonstrated and commercialized. [ 45 ] Another cornerstone of metamaterial research is “transformation optics”, a.k.a. “coordinate transformation”, where the concept of “cloaking [ 46 ] ” has drawn significant attention from the public and academic community.…”
Section: Clustering Abstractmentioning
confidence: 99%