The neutron capture cross sections of 134 Ba, 135 Ba, 136 Ba, and 137 Ba were measured in the energy range from 5 to 225 keV at the Karlsruhe 3.75 MV Van de Graaff accelerator. Neutrons were produced via the 7 Li(p,nfBe reaction by bombarding metallic Li targets with a pulsed proton beam. Capture events were registered with the Karlsruhe 47r Barium Fluoride Detector. Several runs have been performed under different experimental conditions to study the systematic uncertainties, which resulted mainly from the large ratios of total to capture cross sections of up to 400. The cross section ratios were determined with an overall uncertainty of "'3%, an improvement by factors of five to eight compared to existing data. Severe discrepancies were found with respect to previous results. Maxwellian averaged neutron capture cross sections were calculated for thermal energies between kT = 10 ke V and 100 ke V. These stellar cross sections were used in an s-process analysis. For the s-only isotopes 134 Ba and 136 Ba the Nsratio was determined to 0.875±0.025. Hence, a significant brauehing of the s-process path at 134 Cs can be claimed for the first time, in cantrast to predictions from the classical approach. This brauehing yields information on the s-process temperature, indicating values araund T 8 = 2. The new cross sections arealso important for the interpretation of barium isotopic anomalies, which were recently discovered in SiC grains of carbonaceous chondrite meteorites. Tagether with the results from previous experiments on tellurium and samarium, a general improvement of the Nssystematics in the mass range A = 120 to 150 is achieved. This allows for a more reliable separation of s-and r-process yields, resulting in an improved assignment of the respective contributions to eiemental barium that is required for comparison with stellar observations.
ZUSAMMENFASSUNG