free carrier creation and electron-phonon relaxations allowing the dissipation of the laser pulse energy into phonons. [6] For instance, Hudert and co-workers [7] demonstrated that femtosecond pulses are generating coherent acoustic phonons in silicon membranes, the latter phonons being detected by monitoring the changes of the dielectric constant in a pump probe experiment. In 1996, Hase and co-workers demonstrated that such coherent acoustic phonons, generated in a bismuth thin film, are interfering when generated by two delayed pulses. [8] Other experiments on thin films have demonstrated acoustic phonons propagation and reflections in layered media yielding to the determination of their velocity and their energy [7] and the fabrication of multilayered media or phononic crystals offers way of manipulating coherent acoustic phonons. [9] As such ultrafast lasers related techniques are offering a large avenue to study and control phonons at nanoscale in order to establish the design rules for future heat sinks at nanoscale. However, once miniaturization is pushed to its lower limit reaching, standard pump-probe reflection techniques relying on the detection of phonon wave propagation and reflection in thin films [7,8] are not relevant anymore when nanostructure dimensions are of the order of magnitude of optical wavelengths. Alternative approaches are required to investigate the phonons properties of acoustic phonon frequency.To address this bottleneck, we have implemented an alternative approach to probe high frequency phonons up to in the 1 to 20 THz range relying on inelastic scattering spectroscopy coupled to femtosecond pulses. Our approach allows to directly access to the acoustic phonon spectrum, which usually require to collect the time-dependent reflectivity Fourier transform. [7,8] Furthermore, we demonstrate that the temporal and spectral shaping of femtosecond pulses controls this coherent acoustic phonon emission spectrum in silicon metasurfaces.