Lunar maria are filled by massive basaltic lava flows layered one over another, suggesting multiple volcanic eruptions (Hiesinger et al., 2003;Sato et al., 2017;Schaber, 1973). Most exposed mare basalt layers dated from ∼3.8 to 3.1 Ga. Some small-scale volcanisms may continue to 1.2 Ga (Hiesinger et al., 2010). In Imbrium basin, the oldest mare basalt dated from an Apollo sample is 3.5 billion years for Imbrium low-titanium basalt (Heiken et al., 1991). Due to subsequent meteoric impact and space weathering between lava flows (about 1 Ga), the paleoregolith layers will be likely formed and then covered by younger Eratosthenian lava flows (high-titanium) (see Figure 1a; Heiken et al., 1991;Wilhelms, 1987). The depth and thickness of the paleoregolith deposits can provide solid constraints on the volume of lava flows and regolith production rate that are directly associated with meteorite flux during this period. The paleoregolith layers have been undisturbed since their formation thus are critical for determining early impacting and volcano history of the Moon and are regarded as important records for uncovering early Moon's history and early solar system history (