Retrieval of Gridded Aerosol Direct Radiative Forcing Based on Multiplatform Datasets

Abstract

Abstract. Atmospheric aerosols play a crucial role in regional radiative budgets. Previous studies on clear-sky aerosol direct radiative forcing (ADRF) have mainly been limited to site-scale observations or model simulations for short-term cases, and long-term distributions of ADRF in China has not been portrayed yet. In this study, an accurate fine-resolution ADRF estimate at the surface was proposed. Multiplatform datasets, including satellite (Terra and Aqua) and reanalysis datasets, served as inputs to the Santa Barbara Discrete Atmospheric Radiative Transfer (SBDART) model for ADRF simulation with consideration of the aerosol vertical profile over East China during 2000–2016. Specifically, single scattering albedo (SSA) from the Modern-Era Retrospective Analysis for Research and Application, version 2 (MERRA-2) was validated with sunphotometers over East China. The gridded asymmetry parameter (ASY) was then simulated by matching the calculated top-of-atmosphere (TOA) radiative fluxes from the radiative transfer model with satellite observations (Clouds and the Earth's Radiant Energy System (CERES)). The high correlation and small discrepancy (6–8 W m-2) between simulated and observed radiative fluxes at three sites (Baoshan, Fuzhou, and Yong'an) indicated that ADRF retrieval is feasible and has high accuracy over East China. Then this method was applied in each grid of East China and the overall picture of ADRF distributions over East China during 2000–2016 was displayed. ADRF ranges from −220 to −20 W m-2, and annual mean ADRF is −100.21 W m-2, implying that aerosols have strong cooling effect at the surface during past 16 years. Finally, uncertainty analysis was also evaluated. Our method provides the long-term ADRF distribution over East China for the first time, with highlighting the importance of aerosol radiative impact under the climate change.