Retrieval of Aerosol Fine-mode Fraction over China from Satellite Multiangle Polarized Observations: Validation and Application

Abstract

Abstract. The aerosol fine-mode fraction (FMF) is an important optical parameter of aerosols, and the FMF is difficult to accurately retrieve by traditional satellite remote sensing methods. In this study, FMF retrieval was carried out based on the multiangle polarization data of Polarization and Anisotropy of Reflectances for Atmospheric Science coupled with Observations from Lidar (PARASOL), which overcame the shortcomings of the FMF retrieval algorithm in our previous research. In this research, FMF retrieval was carried out in China and compared with the AErosol RObotic NETwork (AERONET) ground-based observation results, Moderate Resolution Imaging Spectroradiometer (MODIS) FMF products, and Generalized Retrieval of Aerosol and Surface Properties (GRASP) FMF results. In addition, application of the FMF retrieval algorithm was carried out, a new FMF dataset was produced, and the annual and quarterly average results of FMF from 2006 to 2013 were obtained in all of China. The research results show that the FMF retrieval results of this study are comparable with the AERONET ground-based observation results in China, with correlation coefficient (r), mean absolute error (MAE), root mean square error (RMSE), and the proportion of results that fall with the expected error (Within EE) are 0.770, 0.143, 0.170, and 60.96 %, respectively. Compared with the MODIS FMF products, the FMF results of this study are closer to the AERONET ground-based observations. Compared with the FMF results of GRASP, the FMF results of this study are closer to the spatial variation in the ratio of PM2.5 to PM10 near the ground. The analysis of the annual and seasonal average FMF of China from 2006 to 2013 shows that the FMF high value area in China is mainly maintained in the area east of the Hu Line, with the highest FMF year being 2013, and the highest FMF season is winter.