1996
DOI: 10.12693/aphyspola.90.519
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Resonant Optical Rectification in Chiral Molecular Systems: Application to a Three-Level Model

Abstract: Α molecular approach to optical rectification via the imaginary part of the second-order susceptibility related to electrie dipole interaction with the radiation freld is presented. Α quantum-mechanical expression for the frequency dependence of the effect is obtained and its magnitude is estimated in absorption bands of a three-level model.PACS numbers: 33.55.Fi, 42.65.ΑrιLinear and nonlinear interactions of an electromagnetic wave with molecules of an isotropic medium induce in them multipole moments which c… Show more

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