2005
DOI: 10.1063/1.1924886
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Remarkable polarization sensitivity of gold nanoparticle arrays

Abstract: In an array of low-symmetry, L-shaped gold nanoparticles, slight distortions of particle shape and arm lengths eliminate the array’s mirror plane. Such asymmetries induce large angular shifts (∼10°) of the resonant extinction axes directions from those of mirror-symmetric particles. The axes directions exhibit dispersion, as allowed by the lack of any structural features dictating them. The nanostructures are chiral, and evidence of optical activity is observed. Rigorous diffraction theory calculations qualita… Show more

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Cited by 58 publications
(41 citation statements)
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“…Using these parameters in conjunction with the analytical expressions for the rearranged constituents as derived below, the optical response of the modified metaatoms can be predicted. The first investigated structure is the L -metaatom 43,44 . In this geometry one of the SRR arms is omitted in order to prevent the cancelation of the far-field that originated from the antiparallel dipole moments.…”
Section: The L -Metaatommentioning
confidence: 99%
“…Using these parameters in conjunction with the analytical expressions for the rearranged constituents as derived below, the optical response of the modified metaatoms can be predicted. The first investigated structure is the L -metaatom 43,44 . In this geometry one of the SRR arms is omitted in order to prevent the cancelation of the far-field that originated from the antiparallel dipole moments.…”
Section: The L -Metaatommentioning
confidence: 99%
“…A conventional approach to studying arrays of nanoobjects deals with optical reflectivity [20,21] or nonlinear-optical conversion [22][23][24], allowing us to find such interesting phenomena as coherent control of optical transmission [25], enhancement of the up-conversion luminescence intensity [26], and periodicity-induced pulse splitting [27]. On the other hand, much less attention is drawn towards polarization effects which are capable of revealing the dynamics of the optical anisotropy induced by a fs laser pulse.…”
Section: Introductionmentioning
confidence: 99%
“…A wide range of even planar chiral plasmonic metamaterials have shown giant chiral interplay with circularly polarized light despite they are not truly chiral. [19][20][21][22][23][24] As a matter of fact, planar chiral metamaterials in the form of a 2D gammadions array have generated superchiral electromagnetic fields offering a strong interaction with chiral materials consisting of biomacromolecules for ultrasensitive characterization. [7] However, as also recently demonstrated by the enhanced chiral optical response of 3D plasmonic nanostructures, [25][26][27][28][29][30][31][32][33][34][35][36][37] chirality is an intrinsic property of 3D objects and, in particular, among the possible 3D chiral shapes, lacking of mirror symmetry, the helical configuration has exhibited large chiral response in the far field.…”
Section: Wwwadvopticalmatdementioning
confidence: 99%