This manuscript has been reproduced from the microfilm master. UMI films the text directly from the original or copy submitted. Thus, some thesis and dissertation copies are in typewriter face, while others may be from any type of computer printer.The quality of this reproduction is dependent upon the quality of the copy submitted. Broken or indistinct print, colored or poor quality illustrations and photographs, print bleedthrough, substandard margins, and improper alignment can adversely affect reproduction.In the unlikely event that the author did not send UMI a complete manuscript and there are missing pages, these will be noted. Also, if unauthorized copyright material had to be removed, a note will indicate the deletion. My primary contact for the cross section generation portion of this project was Robert MacFarlane. His tireless aid through countless phone conversations is appreciated more than he may ever know, and the experience gained through his efforts is invaluable. Having just brushed the surface of an area to which he has dedicated a career has given me an appreciation for the complexity of cross section generation, and has stirred great curiosity and interest.Two groups at Los Alamos National Laboratory have also aided in this project. The Advanced Nuclear Technology Group provided an ideal workplace for my summer Practicum, and much of the concepts developed here began last summer. I would also like to thank Tom MacLaughlin and Doug O'Dell from Criticality Safety for the use of their marvelous CRAY.As an aside, Forrest Brinkley has shown such an interest in helping me with TWODANT whenever there was a question that he had to be mentioned. He truly enjoys helping others, and he does this to a degree which could never expected.The writing of this thesis could not have been accomplished without the unending support of my family. Many sacrifices were made during the exponential portion of the project so that the computer could be available for my use.