“…The closed circles show the magnetization at H decreasing from 50 to À50 kOe and the open circles at H increasing from À 50 to 50 kOe for NaNiF 3 pPv at 2 K. The double loops observed in Fig. 4(g) may be caused by spin flop transition, as interpreted for the double loops in KCuF 3 [37]. Change from antiferromagnetism under low magnetic field to canted antiferromagnetism under high magntic field for NaNiF 3 pPv supports the spin flop transition.…”
Section: Physical Properties Of Nanif 3 Pv and Ppvmentioning
“…The closed circles show the magnetization at H decreasing from 50 to À50 kOe and the open circles at H increasing from À 50 to 50 kOe for NaNiF 3 pPv at 2 K. The double loops observed in Fig. 4(g) may be caused by spin flop transition, as interpreted for the double loops in KCuF 3 [37]. Change from antiferromagnetism under low magnetic field to canted antiferromagnetism under high magntic field for NaNiF 3 pPv supports the spin flop transition.…”
Section: Physical Properties Of Nanif 3 Pv and Ppvmentioning
“…Typically all eight possible antiferromagnetic domains will form within the sample as it is cooled below T N (see fig 2a) so while longitudinal and transverse magnetic excitations can be defined within each domain they cannot be disentangled for the sample as a whole. However, when a magnetic field B, is applied along the crystallographic b direction of KCuF 3 a reorientation of spin moments occurs resulting in a spin-flop phase for fields above 0.8T [25,31]. In this phase the spin moments flop perpendicular to the b direction and due to the x-y anisotropy [22] they point along the a axis [31] resulting in a unique domain throughout the sample (see fig 2b).…”
Section: Polarized Measurementsmentioning
confidence: 99%
“…In zero-field, magnetic order in KCuF 3 is characterised by a structure where spin moments are slightly canted away from the [1,1,0] direction and its symmetry equivalents [23,24,25]. Typically all eight possible antiferromagnetic domains will form within the sample as it is cooled below T N (see fig 2a) so while longitudinal and transverse magnetic excitations can be defined within each domain they cannot be disentangled for the sample as a whole.…”
The spin dynamics of coupled spin-1/2, antiferromagnetic Heisenberg chains is predicted to exhibit a novel longitudinal mode at low energies and temperatures below the Néel temperature. This mode is a dimensional crossover effect and reveals the presence of a limited amount of long-range antiferromagnetic order co-existing with quantum fluctuations. In this paper the existence of such a mode is confirmed in the model material KCuF 3 using polarized and unpolarized inelastic neutron scattering and the longitudinal polarization of the mode is definitively established. The lineshape is broadened suggesting a reduced lifetime due to decay into spin-waves. In addition the data shows evidence of continuum scattering with a lower edge greater than the longitudinal mode energy. A detailed comparison is made with theoretical predictions and experimental work on other model materials.
“…1(a) we show the temperature dependence of the magnetic susceptibility together with a fit obtained by using a rational function which approximates the Bonner-Fisher approach for an antiferromagnetic chain [33,34] traces [35]. The specific heat divided by temperature C/T ( Fig.…”
Section: Experimental Details and Characterizationmentioning
This article is dedicated to Dieter Vollhardt on the occasion of his 60th birthday.We report on polarization dependent reflectivity measurements in KCuF3 in the far-infrared frequency regime. The observed IR active phonons at room temperature are in agreement with the expected modes for tetragonal symmetry. We observe a splitting of one mode already at 150 K and the appearance of a new mode in the vicinity of the Néel temperature.
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