Abstract:Water usage is expected to greatly increase when CO2 capture is added to thermal power plants. A major contribution is the reduction of flue gases temperatures from 100-150 ºC to 30-50 ºC. The majority of studies to date propose the use of direct contact cooling, combining a cold water loop with water cooling. This article expands on a previous study of the same authors [1] proposing dry air-cooled options with rotary regenerative gas/gas heat exchangers, relying on ambient air as the cooling fluid, to elimina… Show more
“…Accordingly, heating reactor plays an important role in achieving fast reaction rates and high energy efficiencies. Conventional reactors are based on radiative heating by electrical furnaces in laboratories or through fuel combustion in industries [1], and include heat transfer process and complicate system with large volumes, leading to large temperature gradient within reactors [2,3]. It needs to be maintained at high temperatures while reactors only occupy a small volume ratio in the system [4,5], which greatly reduces system energy efficiency.…”
Joule-heating reactors have the higher energy efficiency and product selectivity compared with the reactors based on radiative heating. Current Joule-heating reactors are constructed with electrically-conductive metals or carbon materials, and therefore suffer from stability issue due to the presence of corrosive or oxidizing gases during high-temperature reactions. In this study, chemically-stable and electrically-conductive (La0.80Sr0.20)0.95FeO3 (LSF)/Gd0.1Ce0.9O2 (GDC) ceramics have been used to construct Joule-heating reactors for the first time. Taking the advantage of the resistance decrease of the ceramic reactors with temperature increase, the ceramic reactors heated under current control mode achieved the automatic adjustment of heating to stabilize reactor temperatures. In addition, the electrical resistance of LSF/GDC reactors can be tuned by the content of the high-conductive LSF in composite ceramics and ceramic density via sintering temperature, which offers flexibility to control reactor temperatures. The ceramic reactors with dendritic channels (less than 100 µm in diameter) showed the catalytic activity for CO oxidation, which was further improved by coating efficient MnO2 nanocatalyst on reactor channel wall. The Joule-heating ceramic reactors achieved complete CO oxidation at a low temperature of 165 °C. Therefore, robust ceramic reactors have successfully demonstrated effective Joule heating for CO oxidation, which are potentially applied in other high-temperature catalytic reactions.
“…Accordingly, heating reactor plays an important role in achieving fast reaction rates and high energy efficiencies. Conventional reactors are based on radiative heating by electrical furnaces in laboratories or through fuel combustion in industries [1], and include heat transfer process and complicate system with large volumes, leading to large temperature gradient within reactors [2,3]. It needs to be maintained at high temperatures while reactors only occupy a small volume ratio in the system [4,5], which greatly reduces system energy efficiency.…”
Joule-heating reactors have the higher energy efficiency and product selectivity compared with the reactors based on radiative heating. Current Joule-heating reactors are constructed with electrically-conductive metals or carbon materials, and therefore suffer from stability issue due to the presence of corrosive or oxidizing gases during high-temperature reactions. In this study, chemically-stable and electrically-conductive (La0.80Sr0.20)0.95FeO3 (LSF)/Gd0.1Ce0.9O2 (GDC) ceramics have been used to construct Joule-heating reactors for the first time. Taking the advantage of the resistance decrease of the ceramic reactors with temperature increase, the ceramic reactors heated under current control mode achieved the automatic adjustment of heating to stabilize reactor temperatures. In addition, the electrical resistance of LSF/GDC reactors can be tuned by the content of the high-conductive LSF in composite ceramics and ceramic density via sintering temperature, which offers flexibility to control reactor temperatures. The ceramic reactors with dendritic channels (less than 100 µm in diameter) showed the catalytic activity for CO oxidation, which was further improved by coating efficient MnO2 nanocatalyst on reactor channel wall. The Joule-heating ceramic reactors achieved complete CO oxidation at a low temperature of 165 °C. Therefore, robust ceramic reactors have successfully demonstrated effective Joule heating for CO oxidation, which are potentially applied in other high-temperature catalytic reactions.
“…Wang et al [26] developed the thermal hydraulic calculation program integrated with the multi-objective and single-objective genetic algorithms to perform design optimizations of regenerative air preheaters used in the coal-fired power plants. Herraiz et al [27] investigated the use of rotary regenerative heat exchangers for the dry cooling of flue gases in combined cycle gas turbine plants equipped with post-combustion carbon capture. Sheng and Fang [28] experimentally investigated the effect of moisture on the air cleaning performance of a desiccant wheel with the objective to guide practical operation of clear air heat pump.…”
A computational analysis in a rotary regenerative air preheater subject to pre-established mass flow rate is performed. The heat transfer rate, the pressure drop and the outlet temperatures of gas streams are calculated from different matrix porosity values. The fluid flow and the convective heat transfer coefficient are determined from correlations. The total heat transfer is obtained using the Effectiveness-NTU method specific to regenerative air preheaters. Three typical regenerative air preheaters with both streams under the laminar flow regime are investigated. A range of porosity values that provide good thermal exchange and low pressure drop in the equipment is chosen for each examined air preheater. The behavior of the outlet temperatures of each gas stream as function of porosity is also analyzed. The results show that the porosity ranges shorten when the typical pressured drop values for each regenerative air preheater are introduced in the analysis. In addition, the behavior of the outlet temperatures is compatible with the behavior of the heat transfer rate as the porosity changes.
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