Abstract:In this paper, the internal mechanism of solid deuterium spatial distribution induced by infrared radiation is studied. The changes in spatial distribution and micro-structure of solid deuterium are also discussed as the results of wavelength and heating time of IR light. It is found that the micro-structure of solid deuterium which is irradiated by a special IR light is changed from polycrystal to monocrystal, the solid deuterium is redistributed and becomes more uniform and transparent. The best wavelength o… Show more
“…where I 0 is the incident IR light power at x = 0, V is the volume at the position x, and α is the absorption coefficient of the material. In our experiment, the absorption coefficients [12] of solid D 2 and quartz are 1.02 cm −1 and 1.55 cm −1 , respectively. Some intrinsic parameters [14] of solid D 2 and quartz are shown in Table 1.…”
Section: Analysis and Discussionmentioning
confidence: 48%
“…In our previous studies, [12] a strong absorption peak was found at 3140 nm by measuring the IR absorption spectra of liquid D 2 at different temperatures. In the present experiment, the incident IR light is selected to be 3140 nm in wavelength and 100 µW in power.…”
The infrared-induced temperature distributions of solid D 2 ices Bi Peng(毕 鹏) a)b) , Xie Duan(谢 端) a) , Lin Wei(林 伟) a) , Wang Kai(王 凯) a) , Liu Jiang-Ping(刘江平) a)b) , Tang Yong-Jian(唐永建) a) , Yang Xiang-Dong(杨向东) b) , and Lei Hai-Le(雷海乐) a) † a)
“…where I 0 is the incident IR light power at x = 0, V is the volume at the position x, and α is the absorption coefficient of the material. In our experiment, the absorption coefficients [12] of solid D 2 and quartz are 1.02 cm −1 and 1.55 cm −1 , respectively. Some intrinsic parameters [14] of solid D 2 and quartz are shown in Table 1.…”
Section: Analysis and Discussionmentioning
confidence: 48%
“…In our previous studies, [12] a strong absorption peak was found at 3140 nm by measuring the IR absorption spectra of liquid D 2 at different temperatures. In the present experiment, the incident IR light is selected to be 3140 nm in wavelength and 100 µW in power.…”
The infrared-induced temperature distributions of solid D 2 ices Bi Peng(毕 鹏) a)b) , Xie Duan(谢 端) a) , Lin Wei(林 伟) a) , Wang Kai(王 凯) a) , Liu Jiang-Ping(刘江平) a)b) , Tang Yong-Jian(唐永建) a) , Yang Xiang-Dong(杨向东) b) , and Lei Hai-Le(雷海乐) a) † a)
The low mode energy of deuterium is calculated by quantum mechanics theory and deuterium zero-point vibration energy. The smooth, uniformity, euphotic solid deuterium film is obtained by home-made planar cryotarget system. The infrared absorption spectrum of solid deuterium film is studied by infrared spectroscopy system. The strong absorption peaks mostly result from the Q1(0)+S0(0), Q1(0)+S0(1), Q1(0)+S0(0)+S0(1) vibration, rotation modes. The experimental data are in good agreement with the analysis results.
The vibration/rotation modes and the corresponding infrared spectra of deuterium molecules with the D2d/D2h structures are calculated using the coupled cluster singles and doubles method with the cc-PVTZ basis sets within the framework of the density function theory. The infrared (IR) absorption spectrum of liquid deuterium is experimentally measured in a home-made cryogenic target system by a home-made low-temperature infrared spectroscope. The experimental results show that the strongest IR absorption peak of liquid deuterium is related to the Q1(0)+S0(0) mode, which is in good agreement with the theoretical calculation.
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