“…Since the discovery of graphene, layered nanomaterials have been attracted great attention owing to their unique physical properties. , Among them, molybdenum disulfide (MoS 2 ), a semiconducting member of transition metal dichalcogenides (TMDCs), has been extensively investigated in diverse fields of applications due to its fascinating physical, optical, chemical, and catalytic properties. − Interestingly, material quality and related properties can vary based on synthesis methods and significantly affect target-specific application performances. For example, high-quality MoS 2 samples are generally prepared by direct exfoliation from a bulk crystal via micromechanical cleavage ,, or a chemical vapor deposition (CVD) method. − The resulting samples have been used to demonstrate intrinsic properties of MoS 2 for prototype electronic and optoelectronic applications such as transistors, memristors, photosensors, photovoltaic devices, and light-emitting diodes. ,− ,− ,,− However, it is still challenging to translate the proof-of-concepts into practical applications due to the lack of largescale synthesis with high structural and chemical uniformity. In addition, chemical modulation of the constituent atomic compositions is required to generate the best properties of MoS 2 in target-specific applications.…”