2020
DOI: 10.1021/acs.accounts.0c00009 View full text |Buy / Rent full text
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Abstract: Metrics & MoreArticle Recommendations CONSPECTUS: Over the past few years, the development of new materials has contributed to rapid increases in the power conversion efficiencies (PCEs) of organic photovoltaic (OPV) cells to over 17%, showing great potential for the commercialization of this technology in the near future. At this stage, designing new materials with superior performance and low cost simultaneously is of crucial importance. Chlorinated materials are emerging as new stars with very high PCEs, cr… Show more

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“…[7i] It is also interesting to mention that PClBDB-T exhibited red-shift absorption spectra compared to that of PBDB-T-Cl, which should be due to the electronegative effect of Cl atoms. [18] Thef rontier energy levels of JP01 and JP02 were determined by cyclic voltammetry (CV) measurements, as shown in Figure 2b and the Supporting Information, Figure S3. Both of JP01 and JP02 have the similar lowest unoccupied molecular orbital (LUMO) levels with that of the NDI acceptors,while their highest occupied molecular orbital (HOMO) levels are slightly deeper than those of donor polymers (Figure 2b).…”
Section: Synthesis and Characterizationmentioning
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“…[7i] It is also interesting to mention that PClBDB-T exhibited red-shift absorption spectra compared to that of PBDB-T-Cl, which should be due to the electronegative effect of Cl atoms. [18] Thef rontier energy levels of JP01 and JP02 were determined by cyclic voltammetry (CV) measurements, as shown in Figure 2b and the Supporting Information, Figure S3. Both of JP01 and JP02 have the similar lowest unoccupied molecular orbital (LUMO) levels with that of the NDI acceptors,while their highest occupied molecular orbital (HOMO) levels are slightly deeper than those of donor polymers (Figure 2b).…”
Section: Synthesis and Characterizationmentioning
“…significantly increased light absorption and reduced energy losses. [1][2][3][4][5][6] Recently, the PCE of single-junction OSCs is approaching the 18% milestone, exceeding the efficiency threshold expected for industrial viability. [7][8][9][10] Besides efficiency, long-term operational stability, such as thermal-and photostability, is a major concern for the practical application of OSCs.…”
mentioning
“…This unusual phenomenon is absent in the PBI‐based polymer PBDBPBI‐Cl [7i] . It is also interesting to mention that PClBDB‐T exhibited red‐shift absorption spectra compared to that of PBDB‐T‐Cl, which should be due to the electronegative effect of Cl atoms [18] . The frontier energy levels of JP01 and JP02 were determined by cyclic voltammetry (CV) measurements, as shown in Figure 2 b and the Supporting Information, Figure S3.…”
Section: Resultsmentioning