2019
DOI: 10.1007/s40820-019-0335-4
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Recent Progress and Approaches on Carbon-Free Energy from Water Splitting

Abstract: HIGHLIGHTS• Different approaches for efficient carbon-free energy from water splitting are summarized.• Step-wise evolution of water splitting research is highlighted with current progress.• It describes the open challenges of charge transport properties and future research direction.ABSTRACT Sunlight is the most abundant renewable energy resource, providing the earth with enough power that is capable of taking care of all of humanity's desires-a hundred times over. However, as it is at times diffuse and inter… Show more

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Cited by 48 publications
(17 citation statements)
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References 144 publications
(189 reference statements)
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“…Electrochemical water splitting (WS) is considered as a green and convenient method for producing hydrogen (H 2 ) [1][2][3][4]. However, the practical water electrolysis is limited by the sluggish kinetics at cathode (hydrogen evolution reaction, HER) and anode (oxygen evolution reaction, OER) [5][6][7][8][9][10][11]. For industrial WS catalyst, these requirements must be met: (1) stable and high active sites at large current density [12]; (2) continuous intensive gas evolution [13,14]; (3) fast electron transfer [15,16]; (4) low-cost and accessibility [17,18].…”
Section: H O Cmentioning
confidence: 99%
“…Electrochemical water splitting (WS) is considered as a green and convenient method for producing hydrogen (H 2 ) [1][2][3][4]. However, the practical water electrolysis is limited by the sluggish kinetics at cathode (hydrogen evolution reaction, HER) and anode (oxygen evolution reaction, OER) [5][6][7][8][9][10][11]. For industrial WS catalyst, these requirements must be met: (1) stable and high active sites at large current density [12]; (2) continuous intensive gas evolution [13,14]; (3) fast electron transfer [15,16]; (4) low-cost and accessibility [17,18].…”
Section: H O Cmentioning
confidence: 99%
“…Water electrolysis (WE) can convert renewable sources (i.e., solar, wind) into H 2 with clean and high energy density, but the sluggish kinetics of hydrogen and oxygen evolution reaction (HER and OER) at cathode and anode will hinder its efficiency [ 1 4 ]. Although Pt-/Ir-/Ru-based materials are the best choice to accelerate these two half-reactions, the large-scale hydrogen production is still limited by its shortage and high price [ 5 7 ].…”
Section: Introductionmentioning
confidence: 99%
“…The water molecule splitting reaction at the metal oxide surface holds great promise for energy generation applications. Among all other methods of water molecule dissociation, photocatalytic and electrocatalytic splitting of water molecules using sunlight or electricity are the most effective ways to produce hydrogen due to their high sustainability. But low abundance and the high cost of noble metal catalysts and a lot of required energy input limits the practical applications of these technologies. On the other hand, an innovative method for direct water molecule splitting at the metal oxide surface of the hydroelectric cell has been recently reported by Kotnala et al Hydroelectric cell (HEC) splits water molecules at the metal oxide/ferrite surface directly in H + and OH – ions initially by chemidissociation, followed by physidissociation of water molecules onto defect centers.…”
Section: Introductionmentioning
confidence: 99%