Recent advances in the surface modification strategies towards 3D carbon-based hosts for dendrite-free Li/Na/Zn metal anodes

Chen, Chen; Li, Nian Wu; Yu, Le

doi:10.1016/j.enchem.2024.100117

EnergyChem

2024

DOI: 10.1016/j.enchem.2024.100117

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Recent advances in the surface modification strategies towards 3D carbon-based hosts for dendrite-free Li/Na/Zn metal anodes

Chen Chen,

Nian Wu Li,

Le Yu

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Cited by 3 publications

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Hybrid Interface Chemistry Enabling Mixed Conducting via Ultrafast Microwave Polarization Toward Dendrite‐Free Zn Anodes

Chen,

Cao,

Chen

et al. 2024

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Zn metal anodes in aqueous electrolytes suffer from interface issues including uncontrolled dendrite growth and undesired side reactions, resulting in their limited application in terms of short circuits and cell failure. Herein, a hybrid interface chemistry strategy is developed through ultrafast microwave polarization at the skin region of bare Zn. Owing to efficient Joule heating directed by abundant local hot spots at electron valleys, the rapid establishment of a dense interfacial layer can be realized within a minute. Stabilized Zn with suppressed side reactions or surface corrosion is therefore achieved due to the interfacial protection. Importantly, hybrid zincophilic sites involving laterally/vertically interconnected Cu–Zn intermetallic compound and Zn2+‐conductive oxide species ensure mixed charge conducting (denoted as CuHL@Zn), featuring uniformly distributed electric field and boosted Zn2+ diffusion kinetics. As a consequence, CuHL@Zn in symmetric cells affords lifespans of 2800 and 3200 h with ultra‐low polarization voltages (≈19 and 56 mV) at a plating capacity of 1.0 mAh cm−2 for 1 and 5 mA cm−2, respectively. The CuHL@Zn||MnO2 full cell further exhibits cycling stability with a capacity retention of over 80% for 500 cycles at 2 A g−1.

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Hybrid Interface Chemistry Enabling Mixed Conducting via Ultrafast Microwave Polarization Toward Dendrite‐Free Zn Anodes

Chen,

Cao,

Chen

et al. 2024

Small

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Surface fluorination of nickel nanowires enabling LiF-rich nanoscale solid electrolyte interface for stable lithium anodes

Xu,

Yao,

Yuan

et al. 2024

Chemical Engineering Journal

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Curvature-induced strain to realize differential lithiophilicity for selective lithium deposition and stable lithium anode

Jiang,

Pang,

Luo

et al. 2024

Energy Storage Materials

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Recent advances in the surface modification strategies towards 3D carbon-based hosts for dendrite-free Li/Na/Zn metal anodes

Cited by 3 publications

References 163 publications

Hybrid Interface Chemistry Enabling Mixed Conducting via Ultrafast Microwave Polarization Toward Dendrite‐Free Zn Anodes

Hybrid Interface Chemistry Enabling Mixed Conducting via Ultrafast Microwave Polarization Toward Dendrite‐Free Zn Anodes

Surface fluorination of nickel nanowires enabling LiF-rich nanoscale solid electrolyte interface for stable lithium anodes

Curvature-induced strain to realize differential lithiophilicity for selective lithium deposition and stable lithium anode

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