In recent years, AlGaN/GaN technology has shown its rapid development trend, opening a wide range of potential applications for consumer electronics, medical healthcare, and robotics. [9][10][11] However, due to the limitation of growth kinetics, AlGaN/ GaN heterostructures are grown on rigid substrates such as Si, SiC, and sapphire, causing significant difficulty in realizing flexible devices and circuits.Transfer-printing technology has offered a new strategy, of which AlGaN/ GaN heterojunction membranes can be released from the growth substrate and subsequently transferred onto arbitrary substrates. Various approaches have been used to fabricate flexible AlGaN/ GaN HEMTs. [12][13][14][15][16][17][18][19] Conventional transferprinting methods have been summarized and listed in Table 1. For example, Das et al. reported flexible AlGaN/GaN HEMTs, which were released from sapphire substrate by laser lift-off technique. [12] Lesecq et al. demonstrated AlGaN/GaN HEMTs on an adhesive flexible tape by removing the growth substrate via a mechanical lapping and chemical etching process. [14] In addition, Glavin et al. transferred AlGaN/GaN HEMTs to a flexible substrate through h-BN layer-assisted lift-off process and proved a flexible radiofrequency GaN HEMTs. [15] Recently, electrochemical etching was used to release AlGaN/GaN HEMTs from their growth substrates. [18][19] Although these approaches are effective in transferprinting, they exhibit some drawbacks. For instance, laser lift-off and Si substrate etching techniques failed to achieve good uniformity on the backside of AlGaN/GaN heterostructure due to the uneven and whisker-like micropoles. Besides, the Si backside etching was time consuming, which increases the cost. The h-BN layer-assisted lift-off method requires a complex growth process. It is also difficult to grow a uniform large-size h-BN layer, and thus unable to completely peel off the AlGaN/GaN heterostructure. Electrochemical etching is known to destroy the effective area and integrity of the released GaN layers. More importantly, the above-mentioned AlGaN/ GaN HEMTs transfer methods are based on the bonding and debonding process, indicating the placement of individual devices cannot be changed at will. Therefore, it is required to develop a novel transfer-printing method that offers moreThe development of transferrable free-standing semiconductor materials and their heterogeneous integration to arbitrary substrates open up new possibilities in improving device performance, exploring nonconventional manufacturing approaches, and offering a pathway to soft, conformal, and flexible electronics. In this work, flexible AlGaN/GaN high-electron mobility transistors (HEMTs) are demonstrated, which are transfer-printed from AlGaN/GaN on insulator to a flexible substrate using a novel releasing strategy based on the fast, facile, and reliable transfer process. Flexible AlGaN/GaN HEMTs possess good electrical performance such as the maximum saturated drain current density and transconductance of 110 mA mm −1 and ...